

FOLLOWUS
1. Center for Free-Electron Laser Science, Deutsches Elektronen Synchrotron, Notkestrasse 85,Hamburg,Germany,22607
2. Collaborative Innovation Center for IFSA, School of Physics and Astronomy, Shanghai Jiao Tong University,Shanghai,China,200240
3. Department of Physics and The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, Luruper Chaussee 149,Hamburg,Germany,22761
Published:2021,
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DONGFANG ZHANG, TOBIAS KROH, FELIX RITZKOWSKY, et al. THz-Enhanced DC Ultrafast Electron Diffractometer. [J]. Ultrafast science, 2021, 2021(2).
DONGFANG ZHANG, TOBIAS KROH, FELIX RITZKOWSKY, et al. THz-Enhanced DC Ultrafast Electron Diffractometer. [J]. Ultrafast science, 2021, 2021(2). DOI: 10.34133/2021/9848526.
Terahertz- (THz-) based electron manipulation has recently been shown to hold tremendous promise as a technology for manipulating and driving the next generation of compact ultrafast electron sources. Here
we demonstrate an ultrafast electron diffractometer with THz-driven pulse compression. The electron bunches from a conventional DC gun are compressed by a factor of 10 and reach a duration of ~180 fs (FWHM) with 10
000 electrons/pulse at a 1 kHz repetition rate. The resulting ultrafast electron source is used in a proof-of-principle experiment to probe the photoinduced dynamics of single-crystal silicon. The THz-compressed electron beams produce high-quality diffraction patterns and enable the observation of the ultrafast structural dynamics with improved time resolution. These results validate the maturity of THz-driven ultrafast electron sources for use in precision applications.
R. J. D. Miller, “Mapping atomic motions with ultrabright electrons: the chemists’ gedanken experiment enters the lab frame,” Annual Review of Physical Chemistry, vol. 65, no. 1, pp. 583–604, 2014
J. S. Baskin, H. Liu, and A. H. Zewail, “4D multiple-cathode ultrafast electron microscopy,” Proceedings of the National Academy of Sciences of the United States of America, vol. 111, no. 29, pp. 10479–10484, 2014
R. P. Chatelain, V. R. Morrison, C. Godbout, and B. J. Siwick, “Ultrafast electron diffraction with radio-frequency compressed electron pulses,” Applied Physics Letters, vol. 101, no. 8, article 081901, 2012
M. Gao, H. Jean-Ruel, R. R. Cooney, J. Stampe, M. de Jong, M. Harb, G. Sciaini, G. Moriena, and R. J. Dwayne Miller, “Full characterization of RF compressed femtosecond electron pulses using ponderomotive scattering,” Optics Express, vol. 20, no. 11, pp. 12048–12058, 2012
S. Manz, A. Casandruc, D. Zhang, Y. Zhong, R. A. Loch, A. Marx, T. Hasegawa, L. C. Liu, S. Bayesteh, H. Delsim-Hashemi, M. Hoffmann, M. Felber, M. Hachmann, F. Mayet, J. Hirscht, S. Keskin, M. Hada, S. W. Epp, K. Flöttmann, and R. J. D. Miller, “Mapping atomic motions with ultrabright electrons: towards fundamental limits in space-time resolution,” Faraday Discussions, vol. 177, pp. 467–491, 2015
J. Maxson, D. Cesar, G. Calmasini, A. Ody, P. Musumeci, and D. Alesini, “Direct measurement of sub-10 fs relativistic electron beams with ultralow emittance,” Physical Review Letters, vol. 118, no. 15, article 154802, 2017
H. W. Kim, N. A. Vinokurov, I. H. Baek, K. Y. Oang, M. H. Kim, Y. C. Kim, K.-H. H. Jang, K. Lee, S. S. H. Park, S. S. H. Park, J. Shin, J. Kim, F. Rotermund, S. Cho, T. Feurer, and Y. U. Jeong, “Towards jitter-free ultrafast electron diffraction technology,” Nature Photonics, vol. 14, no. 4, pp. 245–249, 2020
T. van Oudheusden, P. L. E. M. Pasmans, S. B. van der Geer, M. J. de Loos, M. J. van der Wiel, and O. J. Luiten, “Compression of subrelativistic space-charge-dominated electron bunches for single-shot femtosecond electron diffraction,” Physical Review Letters, vol. 105, no. 26, article 264801, 2010
P. Baum, “On the physics of ultrashort single-electron pulses for time-resolved microscopy and diffraction,” Chemical Physics, vol. 423, pp. 55–61, 2013
B. J. Siwick, J. R. Dwyer, R. E. Jordan, and R. J. D. Miller, “An atomic-level view of melting using femtosecond electron diffraction,” Science, vol. 302, no. 5649, pp. 1382–1385, 2003
Y. Xiong, K. J. Wilkin, and M. Centurion, “High-resolution movies of molecular rotational dynamics captured with ultrafast electron diffraction,” Physical Review Research, vol. 2, no. 4, article 043064, 2020
M. R. Otto, L. P. Renée de Cotret, M. J. Stern, and B. J. Siwick, “Solving the jitter problem in microwave compressed ultrafast electron diffraction instruments: robust sub-50 fs cavity-laser phase stabilization,” Structural Dynamics, vol. 4, no. 5, article 051101, 2017
A. H. Zewail, “4D ultrafast electron diffraction, crystallography, and microscopy,” Annual Review of Physical Chemistry, vol. 57, no. 1, pp. 65–103, 2006
P. Baum, and A. H. Zewail, “Breaking resolution limits in ultrafast electron diffraction and microscopy,” Proceedings of the National Academy of Sciences, vol. 103, no. 44, pp. 16105–16110, 2006
F. Qi, Z. Ma, L. Zhao, Y. Cheng, W. Jiang, C. Lu, T. Jiang, D. Qian, Z. Wang, W. Zhang, P. Zhu, X. Zou, W. Wan, D. Xiang, and J. Zhang, “Breaking 50 femtosecond resolution barrier in MeV ultrafast electron diffraction with a double bend achromat compressor,” Physical Review Letters, vol. 124, no. 13, article 134803, 2020
C. Kealhofer, W. Schneider, D. Ehberger, A. Ryabov, F. Krausz, and P. Baum, “All-optical control and metrology of electron pulses,” Science, vol. 352, no. 6284, pp. 429–433, 2016
D. Zhang, A. Fallahi, M. Hemmer, X. Wu, M. Fakhari, Y. Hua, H. Cankaya, A.-L. Calendron, L. E. Zapata, N. H. Matlis, and F. X. Kärtner, “Segmented terahertz electron accelerator and manipulator (STEAM),” Nature Photonics, vol. 12, no. 6, pp. 336–342, 2018
D. Zhang, M. Fakhari, H. Cankaya, A.-L. Calendron, N. H. Matlis, and F. X. Kärtner, “Cascaded multicycle terahertz-driven ultrafast electron acceleration and manipulation,” Physical Review X, vol. 10, no. 1, article 011067, 2020
L. Zhao, H. Tang, C. Lu, T. Jiang, P. Zhu, L. Hu, W. Song, H. Wang, J. Qiu, C. Jing, S. Antipov, D. Xiang, and J. Zhang, “Femtosecond relativistic electron beam with reduced timing jitter from THz driven beam compression,” Physical Review Letters, vol. 124, no. 5, article 054802, 2020
E. C. Snively, M. A. K. Othman, M. Kozina, B. K. Ofori-Okai, S. P. Weathersby, S. Park, X. Shen, X. J. Wang, M. C. Hoffmann, R. K. Li, and E. A. Nanni, “Femtosecond compression dynamics and timing jitter suppression in a THz-driven electron bunch compressor,” Physical Review Letters, vol. 124, no. 5, article 054801, 2020
J. A. Fülöp, Z. Ollmann, C. Lombosi, C. Skrobol, S. Klingebiel, L. Pálfalvi, F. Krausz, S. Karsch, and J. Hebling, “Efficient generation of THz pulses with 0.4 mJ energy,” Optics Express, vol. 22, no. 17, pp. 20155–20163, 2014
A. Ryabov, and P. Baum, “Electron microscopy of electromagnetic waveforms,” Science, vol. 353, no. 6297, pp. 374–377, 2016
J. Hebling, G. Almasi, I. Kozma, and J. Kuhl, “Velocity matching by pulse front tilting for large area THz-pulse generation,” Optics Express, vol. 10, no. 21, pp. 1161–1166, 2002
W. K. H. Panofsky, and W. A. Wenzel, “Some considerations concerning the transverse deflection of charged particles in radio-frequency fields,” The Review of Scientific Instruments, vol. 27, no. 11, p. 967, 1956
CST–Computer Simulation Technology, https://www.cst.com/.
T. van Oudheusden, E. F. de Jong, S. B. van der Geer, W. P. E. M. O. ’t Root, O. J. Luiten, and B. J. Siwick, “Electron source concept for single-shot sub-100 fs electron diffraction in the 100 keV range,” Journal of Applied Physics, vol. 102, no. 9, article 093501, 2007
L. Waldecker, T. Vasileiadis, R. Bertoni, R. Ernstorfer, T. Zier, F. H. Valencia, M. E. Garcia, and E. S. Zijlstra, “Coherent and incoherent structural dynamics in laser-excited antimony,” Physical Review B, vol. 95, no. 5, article 054302, 2017
V. R. Morrison, R. P. Chatelain, K. L. Tiwari, A. Hendaoui, A. Bruhács, M. Chaker, and B. J. Siwick, “A photoinduced metal-like phase of monoclinic VO2 revealed by ultrafast electron diffraction,” Science, vol. 346, no. 6208, pp. 445–448, 2014
H. Çankaya, A.-L. Calendron, C. Zhou, S.-H. Chia, O. D. Mücke, G. Cirmi, and F. X. Kärtner, “40-μJ passively CEP-stable seed source for ytterbium-based high-energy optical waveform synthesizers,” Optics Express, vol. 24, no. 22, pp. 25169–25180, 2016
D. Zhang, A. Fallahi, M. Hemmer, H. Ye, M. Fakhari, Y. Hua, H. Cankaya, A.-L. Calendron, L. E. Zapata, N. H. Matlis, and F. X. Kärtner, “Femtosecond phase control in high-field terahertz-driven ultrafast electron sources,” Optica, vol. 6, no. 7, p. 872, 2019
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