Air-Laser-Based Standoff Coherent Raman Spectrometer

Yao Fu; Jincheng Cao; Kaoru Yamanouchi; Huailiang Xu

doi:10.34133/2022/9867028

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Air-Laser-Based Standoff Coherent Raman Spectrometer

Research Article | Updated：2024-10-22

- Air-Laser-Based Standoff Coherent Raman Spectrometer
- 超快科学（英文） 2022年2卷第4期
- Affiliations：
  
  a State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, Changchun 130012, Chinab Department of Chemistry, School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japanc CAS Center for Excellence in Ultra-Intense Laser Science,Shanghai,China,201800
- Author bio：
- Funds：
  
  The work is supported in part by the National Natural Science Foundation of China (NSFC) (62027822) and Japan Society for the Promotion of Science KAKENHI Grants (15H05696 and 20H00371).
- DOI：10.34133/2022/9867028
  中图分类号：
- 纸质出版日期：2022，
- Accepted：
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Yao Fu, Jincheng Cao, Kaoru Yamanouchi, Huailiang Xu. 2022: Air-Laser-Based Standoff Coherent Raman Spectrometer. 超快科学, 2022(4).

Yao Fu, Jincheng Cao, Kaoru Yamanouchi, Huailiang Xu. 2022: Air-Laser-Based Standoff Coherent Raman Spectrometer. Ultrafast Science, 2022(4).
Yao Fu, Jincheng Cao, Kaoru Yamanouchi, Huailiang Xu. 2022: Air-Laser-Based Standoff Coherent Raman Spectrometer. 超快科学, 2022(4). DOI： 10.34133/2022/9867028

Yao Fu, Jincheng Cao, Kaoru Yamanouchi, Huailiang Xu. 2022: Air-Laser-Based Standoff Coherent Raman Spectrometer. Ultrafast Science, 2022(4). DOI： 10.34133/2022/9867028

摘要

Among currently available optical spectroscopic methods

Raman spectroscopy has versatile application to investigation of dynamical processes of molecules leading to chemical changes in the gas and liquid phases. However

it is still a challenge to realize an ideal standoff coherent Raman spectrometer with which both high temporal resolution and high-frequency resolution can be achieved

so that one can remotely probe chemical species in real time with high temporal resolution while monitoring the populations in their respective rovibronic levels in the frequency domain with sufficiently high spectral resolution. In the present study

we construct an air-laser-based Raman spectrometer

in which near-infrared femtosecond (fs) laser pulses at 800 nm and cavity-free picosecond N2+ air-laser pulses at 391 nm generated by the filamentation induced by the fs laser pulses are simultaneously used

enabling us to generate a hybrid ps/fs laser source at a desired standoff position for standoff surveillance of chemical and biochemical species. With this prototype Raman spectrometer

we demonstrate that the temporal evolution of the electronic

vibrational

and rotational states of N2+ and the coupling processes of the rovibrational wave packet of N2 molecules can be probed.

Abstract

Among currently available optical spectroscopic methods

Raman spectroscopy has versatile application to investigation of dynamical processes of molecules leading to chemical changes in the gas and liquid phases. However

it is still a challenge to realize an ideal standoff coherent Raman spectrometer with which both high temporal resolution and high-frequency resolution can be achieved

we construct an air-laser-based Raman spectrometer

enabling us to generate a hybrid ps/fs laser source at a desired standoff position for standoff surveillance of chemical and biochemical species. With this prototype Raman spectrometer

we demonstrate that the temporal evolution of the electronic

vibrational

and rotational states of N2+ and the coupling processes of the rovibrational wave packet of N2 molecules can be probed.

关键词

Air lasingnitrogen moleculesfemtosecond laserfilamentationRaman Spectroscopy

Keywords

Air lasingnitrogen moleculesfemtosecond laserfilamentationRaman Spectroscopy

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