Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems

doi:10.34133/ultrafastscience.0004

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Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems

Research Article | Updated：2024-10-22

- Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems
- 超快科学（英文） 2023年3卷第4期
- Affiliations：
  
  a ICFO - Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Castelldefels08860, Barcelona, Spain. b Linac Coherent Light Source, SLAC National Accelerator Laboratory,Menlo Park, CA 94025, USA. c European XFEL, Holzkoppel 4, 22869 Schenefeld, Germany. d Institut für Nanophotonik Göttingen e.V., Hans-Adolf-Krebs-Weg 1, 37077 Göttingen, Germany. e Deutsches Elektronen-Synchrotron, Notkestraße 85, 22607 Hamburg, Germany. f Max-Planck-Institut für Struktur und Dynamik der Materie, 22761 Hamburg, Germany. g ICREA, Pg. Lluís Companys 23, 08010 Barcelona,Spain
- Author bio：
- Funds：
- DOI：10.34133/ultrafastscience.0004
  中图分类号：
- 纸质出版日期：2023，
- Accepted：
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Adam M. Summers, Stefano Severino, Maurizio Reduzzi, Themistoklis P. H. Sidiropoulos, Daniel E. Rivas, Nicola Di Palo, Hung-Wei Sun, Ying-Hao Chien, Iker León, Bárbara Buades, Seth L. Cousin, Stephan M. Teichmann, Tobias Mey, Klaus Mann, Barbara Keitel, Elke Plönjes, Dmitri K. Efetov, Heinrich Schwoerer, and Jens Biegert. 2023: Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems. 超快科学, 3(4).

2023: Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems. Ultrafast Science, 3(4).
Adam M. Summers, Stefano Severino, Maurizio Reduzzi, Themistoklis P. H. Sidiropoulos, Daniel E. Rivas, Nicola Di Palo, Hung-Wei Sun, Ying-Hao Chien, Iker León, Bárbara Buades, Seth L. Cousin, Stephan M. Teichmann, Tobias Mey, Klaus Mann, Barbara Keitel, Elke Plönjes, Dmitri K. Efetov, Heinrich Schwoerer, and Jens Biegert. 2023: Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems. 超快科学, 3(4). DOI： 10.34133/ultrafastscience.0004

2023: Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems. Ultrafast Science, 3(4). DOI： 10.34133/ultrafastscience.0004

摘要

Unraveling the exact nature of nonequilibrium and correlated interactions is paramount for continued progress in many areas of condensed matter science. Such insight is a prerequisite to develop an engineered approach for smart materials with targeted properties designed to address standing needs such as efficient light harvesting

energy storage

or information processing. For this goal

it is critical to unravel the dynamics of the energy conversion processes between carriers in the earliest time scales of the excitation dynamics. We discuss the implementation and benefits of attosecond soft x-ray core-level spectroscopy up to photon energies of 600 eV for measurements in solid-state systems.In particular

we examine how the pairing between coherent spectral coverage and temporal resolution provides a powerful new insight into the quantum dynamic interactions that determine the macroscopic electronic and optical response. We highlight the different building blocks of the methodology and point out the important aspects for its application from condensed matter studies to materials as thin as 25 nm. Furthermore

we discuss the technological developments in the field of tabletop attosecond soft x-ray sources with time-resolved measurements at the near and extended edge simultaneously and investigate the exciting prospective of extending such technique to the study of 2-dimensional materials.

Abstract

energy storage

or information processing. For this goal

关键词

attosecond scienceCore-level x-ray SpectroscopyHigh Harmonic GenerationX-ray AbsorptionUltrafast solid-state dynamics

Keywords

attosecond scienceCore-level x-ray SpectroscopyHigh Harmonic GenerationX-ray AbsorptionUltrafast solid-state dynamics

references

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Popova-Gorelova, D.. Perspective: towards real-time extreme ultraviolet to x-ray imaging and spectroscopy of laser-driven materials. Journal of Physics B: Atomic, Molecular and Optical Physics, 2024, 57(17): 172501. DOI:10.1088/1361-6455/ad5fd4.

Severino, S., Ziems, K.M., Reduzzi, M. et al. Attosecond core-level absorption spectroscopy reveals the electronic and nuclear dynamics of molecular ring opening. Nature Photonics, 2024, 18(7): 731-737. DOI:10.1038/s41566-024-01436-9.

Chen, L.X., Yano, J. Deciphering Photoinduced Catalytic Reaction Mechanisms in Natural and Artificial Photosynthetic Systems on Multiple Temporal and Spatial Scales Using X-ray Probes. Chemical Reviews, 2024, 124(9): 5421-5469. DOI:10.1021/acs.chemrev.3c00560.

Di Palo, N., Inzani, G., Dolso, G.L. et al. Attosecond absorption and reflection spectroscopy of solids. APL Photonics, 2024, 9(2): 020901. DOI:10.1063/5.0176656.

Biegert, J.. ATTOSECOND SCIENCE: A NEW ERA FOR MANY-BODY PHYSICS. Europhysics News, 2024, 55(1): 12-15. DOI:10.1051/epn/2024105.

Garratt, D., Matthews, M., Marangos, J. Toward ultrafast soft x-ray spectroscopy of organic photovoltaic devices. Structural Dynamics, 2024, 11(1): 010901. DOI:10.1063/4.0000214.

Sidiropoulos, T.P.H., Di Palo, N., Rivas, D.E. et al. Enhanced optical conductivity and many-body effects in strongly-driven photo-excited semi-metallic graphite. Nature Communications, 2023, 14(1): 7407. DOI:10.1038/s41467-023-43191-5.

Li, J., Liu, Y. Hearing the Heartbeat of Atoms: Unveiling Attosecond Horizons. Ultrafast Science, 2023. DOI:10.34133/ultrafastscience.0049.

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